37722 - Experimental Methodologies for the Preparation of Drugs (GR_A)

Academic Year 2014/2015

  • Docente: Alberto Leoni
  • Credits: 10
  • Language: Italian
  • Teaching Mode: In-person learning (entirely or partially)
  • Campus: Bologna
  • Corso: Single cycle degree programme (LMCU) in Chemistry and Pharmaceutical Technologies (cod. 8412)

Learning outcomes

THE COURSE PROVIDES AN INTRODUCTION TO VARIOUS TECHNIQUES OF SYNTHESIS AND EXTRACTION OF COMPOUNDS OF PHARMACEUTICAL INTEREST. MAJOR OBJECTIVES OF COURSE ARE IMPROVEMENT OF SKILL IN THE TECHNICAL ASPECTS OF LABORATORY WORK (I.E. SAFE HANDLING OF CHEMICALS, APPARATUS MANIPULATION) AND INTRODUCTION TO TECHNIQUES AND PROCEDURES IMPORTANT TO THE SUCCESSFUL PRACTICE OF EXPERIMENTS

Course contents

Theoretical lessons
General instructions for safe working in organical chemical laboratories.
Apparatus and reaction procedures: glassware, apparatus with interchangeable ground glass joints suitable for general use in preparative organic chemistry: care and maintenance. Cooling and heating of reaction mixtures. Mechanical agitation.
Isolation and purification processes: Solids purification. Decolouration. Filtration techniques: filter funnels and membrane filters. Recrystallisation tecniques. Extraction theory. Solvent extraction. Countercurrent extraction: Craig apparatus. Solid phase extraction. Drying of solids and apparatus. Anhydrous reactions. Drying of liquids or of solutions of organic compounds in organic solvents: drying agents. Distillation. Rotary evaporator. Steam distillation. Fractional distillation at atmospheric and diminished pressure. Molecular distillation. Purification of common organic solvents. Silica gel column chromatography: flash chromatography.
Microwave-assisted synthesis of pharmaceutical compounds
Combinatorial chemistry in drug discovery. Solid phase synthesis
.
Some novel and common oxidizing and reducing agents.
Extraction, biosynthesis, and chemical synthesis of pharmaceutical compounds
: taxol, camptothecin, erythromycine, epibatidine, philanthotoxins.
Guidelines for Keeping a Laboratory Record.
Practical laboratory:
- Enantioselective enzymatic reduction of methylacetoacetate and purification by gravity-flow column chromatography.
-N-BOC protection of proline.
-Synthesis of tacrine.
-Synthesis of trans-9-(2-phenylethenyl)anthracene.
-Synthesis of nifedipine.
-Oxidation of isoborneol to camphor by potassium chromate.
-Reduction of camphor to isoborneol by sodium borohydride.
-Synthesis of p-nitroacetanilide and purification by flash chromatography.
-Synthesis of acetylsalicylic acid.
-Resolution of racemic 1-phenylethylamine by fractional crystallization.
-Extraction, purification and quantitative determination of beta-carotene from Lycospericon Esculentum
-Extraction and separation of hibiscus acid, hibiscin and caffeic acid from dried calyces of Hibiscus Sabdariffa by Extralut column.
-Extraction of trimyristine from Myristica Fragrans.
-Extraction of eugenol by steam distillation from Syzygium Aromaticum.
- Extraction of flavonoids and essential oil from dried flowers of Matricaria Camomilla.
- Extraction and quantitative determination of nicotine fron dried leaves of Nicotiana Tabaccum.
- Solid phase extraction and quantitative determination of xanthines from dried leaves of Thea Sinensis. 

Readings/Bibliography

1) VOGEL. CHIMICA ORGANICA PRATICA. CASA EDITRICE AMBROSIANA, SECONDA EDIZIONE, MILANO 1988 2) R. M. ROBERTS, J.C. GILBERT, S. F. MARTIN. CHIMICA ORGANICA SPERIMENTALE. ZANICHELLI, BOLOGNA 2003 3) A.J. HANDELY. EXTRACTION METHODS IN ORGANIC ANALYSIS. SHEFFIELD ACADEMIC PRESS, CANADA 1999 4) D.L. PAVIA, G. M. LAMPMAN, G.S. KRIZ. IL LABORATORIO DI CHIMICA ORGANICA, EDIZIONI SORBONA , MILANO 1994 5) P.M. DEWICK. CHIMICA, BIOSINTESI E BIOATTIVITA' DELLE SOSTANZE NATURALI. PICCIN, PADOVA 2000 6) MARCO D'ISCHIA LA CHIMICA ORGANICA IN LABORATORIO PICCIN PADOVA 2002

Teaching methods

The course will be supported by laboratory exercises. The
laboratory exercises will be individual and will aim to
provide each student the opportunity to apply the various
methods of preparing extracts of herbal drugs outlined
in theoretical form in class.

Assessment methods

FINAL EXAMINATION:
A comprehensive final exam is given at the end of the semester. The final test will tend to determine the knowledge of the topics presented during the lessons.

Teaching tools

PC, LABORATORY OF CHEMISTRY, TRASPARENCIES, VIDEOPROJECTORS

Office hours

See the website of Alberto Leoni